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User authentication systems based on cardiovascular biosignals have gained prominence in recent years, as these signals are presumed to be difficult to forge. We challenge this assumption by showing that an observer who has access to one type of cardiac data --- such as a user's pulse waveform, readily obtainable from video and commercial smartwatches --- can design a spoofing attack strong enough to fool authentication systems based on other cardiovascular biosignals. We present BioForge, an approach that leverages a cycle-consistent generative adversarial network to synthesize realistic physiological signals for a given user without relying on simultaneously collected supervision data. We evaluate BioForge on multiple open-access datasets and an array of verification systems, many of which can be fooled over 50% of the time in 10 or fewer attempts. Notably, we are able to fool systems that rely not just on heart rate and peak locations but also on the morphology of the waveforms. We additionally showcase how BioForge can be used to spoof authentication systems from biosignal data extracted from video clips of a target user. Our work demonstrates that authentication systems should not rely on the secrecy of cardiovascular biosignals. 

We present a modular approach to reinforcement learning (RL) in environments consisting of simpler components evolving in parallel. A monolithic view of such modular environments may be prohibitively large to learn, or may require unrealizable communication between the components in the form of a centralized controller. Our proposed approach is based on the assume-guarantee paradigm where the optimal control for the individual components is synthesized in isolation by making assumptions about the behaviors of neighboring components, and providing guarantees about their own behavior. We express these assume-guarantee contracts as regular languages and provide automatic translations to scalar rewards to be used in RL. By combining local probabilities of satisfaction for each component, we provide a lower bound on the probability of sat- isfaction of the complete system. By solving a Markov game for each component, RL can produce a controller for each component that maximizes this lower bound. The controller utilizes the information it receives through communication, observations, and any knowledge of a coarse model of other agents. We experimentally demonstrate the efficiency of the proposed approach on a variety of case studies. 

We report on the use of extreme ultraviolet (XUV, 30.3 nm) radiation from the Free-electron LASer in Hamburg (FLASH) and visible (Vis, 405 nm) photons from an optical laser to investigate the relaxation and fragmentation dynamics of fluorene ions. The ultrashort laser pulses allow to resolve the molecular processes occurring on the femtosecond timescales. Fluorene is a prototypical small polycyclic aromatic hydrocarbon (PAH). Through their infrared emission signature, PAHs have been shown to be ubiquitous in the universe, and they are assumed to play an important role in the chemistry of the interstellar medium. Our experiments track the ionization and dissociative ionization products of fluorene through time-of-flight mass spectrometry and velocity-map imaging. Multiple processes involved in the formation of each of the fragment ions are disentangled through analysis of the ion images. The relaxation lifetimes of the excited fluorene monocation and dication obtained through the fragment formation channels are reported to be in the range of a few tens of femtoseconds to a few picoseconds. 

Abstract Polycyclic aromatic hydrocarbons (PAHs) play an important role in interstellar chemistry and are subject to high energy photons that can induce excitation, ionization, and fragmentation. Previous studies have demonstrated electronic relaxation of parent PAH monocations over 10–100 femtoseconds as a result of beyond-Born-Oppenheimer coupling between the electronic and nuclear dynamics. Here, we investigate three PAH molecules: fluorene, phenanthrene, and pyrene, using ultrafast XUV and IR laser pulses. Simultaneous measurements of the ion yields, ion momenta, and electron momenta as a function of laser pulse delay allow a detailed insight into the various molecular processes. We report relaxation times for the electronically excited PAH * , PAH +* and PAH 2+* states, and show the time-dependent conversion between fragmentation pathways. Additionally, using recoil-frame covariance analysis between ion images, we demonstrate that the dissociation of the PAH 2+ ions favors reaction pathways involving two-body breakup and/or loss of neutral fragments totaling an even number of carbon atoms.